@article{Li2021-12-14Bioin-57255,
  year={2021},
  doi={10.1021/acs.chemmater.1c02868},
  title={Bioinspired Compartmentalization Strategy for Coating Polymers with Self-Organized Prismatic Films},
  number={23},
  volume={33},
  issn={0897-4756},
  journal={Chemistry of Materials},
  pages={9240--9251},
  author={Li, Zheng-Zheng and Li, Ming and Feng, Yu-xuan and Zhang, Zhisen and Wen, Yue-E and Huang, Qi-Qi and Cölfen, Helmut and Fratzl, Peter and Amini, Shahrouz and Jiang, Yuan}
}

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    <dc:creator>Cölfen, Helmut</dc:creator>
    <dc:contributor>Li, Ming</dc:contributor>
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    <dc:contributor>Wen, Yue-E</dc:contributor>
    <dcterms:issued>2021-12-14</dcterms:issued>
    <dc:language>eng</dc:language>
    <dc:creator>Fratzl, Peter</dc:creator>
    <dc:creator>Wen, Yue-E</dc:creator>
    <dc:contributor>Jiang, Yuan</dc:contributor>
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    <dc:contributor>Cölfen, Helmut</dc:contributor>
    <dc:creator>Huang, Qi-Qi</dc:creator>
    <dc:creator>Amini, Shahrouz</dc:creator>
    <dc:contributor>Feng, Yu-xuan</dc:contributor>
    <dc:contributor>Huang, Qi-Qi</dc:contributor>
    <dc:creator>Li, Ming</dc:creator>
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    <dc:contributor>Li, Zheng-Zheng</dc:contributor>
    <dc:creator>Zhang, Zhisen</dc:creator>
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    <dc:creator>Feng, Yu-xuan</dc:creator>
    <dc:contributor>Zhang, Zhisen</dc:contributor>
    <dc:contributor>Fratzl, Peter</dc:contributor>
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    <dcterms:title>Bioinspired Compartmentalization Strategy for Coating Polymers with Self-Organized Prismatic Films</dcterms:title>
    <dc:creator>Li, Zheng-Zheng</dc:creator>
    <dc:contributor>Amini, Shahrouz</dc:contributor>
    <dc:creator>Jiang, Yuan</dc:creator>
    <dcterms:abstract xml:lang="eng">Biomineralization provides load-bearing and protective functions to living organisms by reinforcing soft tissues. Translation of biomineralization principles to materials science in a controlled and self-organized fashion is highly desirable but challenging. A major lesson from natural systems is that crystallization may be controlled by compartmentalization and templating. Here, we develop a crystallization technique based on graphene oxide-mediated compartmentalization and on templating prismatic growth of calcite nanocoatings via control of ionic diffusivity into the microcompartments, which results in a multistage, self-organized crystallization and represents an effective strategy for providing continuous nanocoatings and enhancing the tribological performance of polymeric surfaces under contact stresses. The present research offers a bottom-up approach of using very basic biomineralization principles for the protection of polymeric surfaces, which are of interest for biomedical applications and the fabrication of high-performance functional materials in a sustainable manner.</dcterms:abstract>
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