Biquadratic exchange and critical behaviour in the diluted antiferromagnet Eu-Sr-Te

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1993
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Köbler, Ulrich
Apfelstedt, I.
Fischer, K.
Zinn, W.
Wosnitza, Jochen
Löhneysen, Hilbert von
Brückel, Thomas
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Zeitschrift für Physik / B. 1993, 92(4), pp. 475-487. Available under: doi: 10.1007/BF01320511
Zusammenfassung

Magnetization, specific heat, magnetocaloric effect, and neutron diffraction measurements have been performed in order to better understand the magnetic interactions and phase transitions in the diluted antiferromagnetic system EuxSrl_xTe. Due to the low N6el temperature of TN=9.8 K and the associated small critical field of Be(T= 0)= 7.5 T, EuTe provides the opportunity to change the angle between the antiferromagnetic moments continuously between 180 ~ and 0 ~ by applying a magnetic field and allows thus to probe the type of the magnetic interaction. It is found that in addition to the common bilinear Heisenberg exchange mechanism there is evidence for a small biquadratic exchange term, which has important consequences on the critical behaviour of EuxSr~_xTe. In the case of EuTe the biquadratic exchange supports the antiferromagnetic order, such that virtually no anisotropy exists and this restricts the antiferromagnetic (AF) to spin-flop (SF) transition to B0 = 0. On dilution with strontium, the biquadratic interaction decreases strongly and changes its sign at x~0.83 thus favouring the perpendicular moment orientation. This acts like an anisotropy on the dominating antiferromagnetic bilinear interaction and shifts the AF-SF phase line to finite fields which reach values of 0.3 T for T~ 0. No bicritieal behaviour is observed, but instead, the SF phase is the state of lowest energy in a small temperature interval below TN. The critical exponent ~(x) of the specific heat decreases in a non-linear way with dilution starting from a large positive value for EuTe. e(x) is close to the Heisenberg value -0.12 near x~0.83 where the biquadratic interaction is zero. The same applies for the exponent fl of the sublattice magnetization.

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ISO 690KÖBLER, Ulrich, I. APFELSTEDT, K. FISCHER, W. ZINN, Elke SCHEER, Jochen WOSNITZA, Hilbert von LÖHNEYSEN, Thomas BRÜCKEL, 1993. Biquadratic exchange and critical behaviour in the diluted antiferromagnet Eu-Sr-Te. In: Zeitschrift für Physik / B. 1993, 92(4), pp. 475-487. Available under: doi: 10.1007/BF01320511
BibTex
@article{Kobler1993Biqua-8968,
  year={1993},
  doi={10.1007/BF01320511},
  title={Biquadratic exchange and critical behaviour in the diluted antiferromagnet Eu-Sr-Te},
  number={4},
  volume={92},
  journal={Zeitschrift für Physik / B},
  pages={475--487},
  author={Köbler, Ulrich and Apfelstedt, I. and Fischer, K. and Zinn, W. and Scheer, Elke and Wosnitza, Jochen and Löhneysen, Hilbert von and Brückel, Thomas}
}
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