Jenni, K., Wirth, F., Dietrich, K., Berger, L., Sidis, Y., Kunkemoeller, S., Grams, C. P., Khomskii, D., I, Hemberger, J. and Braden, M. (2020). Evidence for current-induced phase coexistence in Ca2RuO4 and its influence on magnetic order. Phys. Rev. Mater., 4 (8). COLLEGE PK: AMER PHYSICAL SOC. ISSN 2475-9953

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Abstract

Combining quasistatic and time-resolved transport measurements with x-ray and neutron diffraction experiments we study the nonequilibrium states that arise in pure and in Ti-substituted Ca2RuO4 under the application of current densities. Time-resolved studies of the current-induced switching find a slow conductance relaxation that can be identified with heating and a fast one that unambiguously proves an intrinsic mechanism. The current-induced phase transition leads to complex diffraction patterns. Separated Bragg reflections that can be associated with the metallic and insulating phases by their lattice parameters, indicate a real structure with phase coexistence that strongly varies with temperature and current strength. A third contribution with a c lattice constant in between those of metallic and insulating phases appears upon cooling. At low current densities, this additional phase appears below similar to 100 K and is accompanied by a suppression of the antiferromagnetic order that otherwise can coexist with current carrying states. A possible origin of the intermediate phase is discussed.

Item Type: Journal Article
Creators:
CreatorsEmailORCIDORCID Put Code
Jenni, K.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Wirth, F.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Dietrich, K.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Berger, L.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Sidis, Y.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Kunkemoeller, S.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Grams, C. P.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Khomskii, D., IUNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Hemberger, J.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
Braden, M.UNSPECIFIEDUNSPECIFIEDUNSPECIFIED
URN: urn:nbn:de:hbz:38-324029
DOI: 10.1103/PhysRevMaterials.4.085001
Journal or Publication Title: Phys. Rev. Mater.
Volume: 4
Number: 8
Date: 2020
Publisher: AMER PHYSICAL SOC
Place of Publication: COLLEGE PK
ISSN: 2475-9953
Language: English
Faculty: Unspecified
Divisions: Unspecified
Subjects: no entry
Uncontrolled Keywords:
KeywordsLanguage
METAL-INSULATOR-TRANSITION; MOTT INSULATORS; CRYSTAL; VO2Multiple languages
Materials Science, MultidisciplinaryMultiple languages
URI: http://kups.ub.uni-koeln.de/id/eprint/32402

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