Research Update : Behind the high efficiency of hybrid perovskite solar cells

Lade...
Vorschaubild
Dateien
Fakharuddin_0-372166.pdf
Fakharuddin_0-372166.pdfGröße: 2.55 MBDownloads: 317
Datum
2016
Autor:innen
De Rossi, Francesca
Watson, Trystan M.
Jose, Rajan
Herausgeber:innen
Kontakt
ISSN der Zeitschrift
Electronic ISSN
ISBN
Bibliografische Daten
Verlag
Schriftenreihe
Auflagebezeichnung
DOI (zitierfähiger Link)
ArXiv-ID
Internationale Patentnummer
Link zur Lizenz
Angaben zur Forschungsförderung
Projekt
Open Access-Veröffentlichung
Open Access Gold
Sammlungen
Core Facility der Universität Konstanz
Gesperrt bis
Titel in einer weiteren Sprache
Forschungsvorhaben
Organisationseinheiten
Zeitschriftenheft
Publikationstyp
Zeitschriftenartikel
Publikationsstatus
Published
Erschienen in
APL Materials. 2016, 4(9), 091505. eISSN 2166-532X. Available under: doi: 10.1063/1.4962143
Zusammenfassung

Perovskite solar cells (PSCs) marked tremendous progress in a short period of time and offer bright hopes for cheap solar electricity. Despite high power conversion efficiency >20%, its poor operational stability as well as involvement of toxic, volatile, and less-abundant materials hinders its practical deployment. The fact that degradation and toxicity are typically observed in the most successful perovskite involving organic cation and toxic lead, i.e., CH3NH3PbX3, requires a deep understanding of their role in photovoltaic performance in order to envisage if a non-toxic, stable yet highly efficient device is feasible. Towards this, we first provide an overview of the basic chemistry and physics of halide perovskites and its correlation with its extraordinary properties such as crystal structure, bandgap, ferroelectricity, and electronic transport. We then discuss device related aspects such as the various device designs in PSCs and role of interfaces in origin of PV parameters particularly open circuit voltage, various film processing methods and their effect on morphology and characteristics of perovskite films, and the origin and elimination of hysteresis and operational stability in these devices. We then identify future perspectives for stable and efficient PSCs for practical deployment.

Zusammenfassung in einer weiteren Sprache
Fachgebiet (DDC)
530 Physik
Schlagwörter
high efficiency, hybrid, perovskite, solar cells
Konferenz
Rezension
undefined / . - undefined, undefined
Zitieren
ISO 690FAKHARUDDIN, Azhar, Francesca DE ROSSI, Trystan M. WATSON, Lukas SCHMIDT-MENDE, Rajan JOSE, 2016. Research Update : Behind the high efficiency of hybrid perovskite solar cells. In: APL Materials. 2016, 4(9), 091505. eISSN 2166-532X. Available under: doi: 10.1063/1.4962143
BibTex
@article{Fakharuddin2016-09-06Resea-35965,
  year={2016},
  doi={10.1063/1.4962143},
  title={Research Update : Behind the high efficiency of hybrid perovskite solar cells},
  number={9},
  volume={4},
  journal={APL Materials},
  author={Fakharuddin, Azhar and De Rossi, Francesca and Watson, Trystan M. and Schmidt-Mende, Lukas and Jose, Rajan},
  note={Article Number: 091505}
}
RDF
<rdf:RDF
    xmlns:dcterms="http://purl.org/dc/terms/"
    xmlns:dc="http://purl.org/dc/elements/1.1/"
    xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#"
    xmlns:bibo="http://purl.org/ontology/bibo/"
    xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#"
    xmlns:foaf="http://xmlns.com/foaf/0.1/"
    xmlns:void="http://rdfs.org/ns/void#"
    xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > 
  <rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/35965">
    <foaf:homepage rdf:resource="http://localhost:8080/"/>
    <dc:rights>Attribution 4.0 International</dc:rights>
    <dc:contributor>Fakharuddin, Azhar</dc:contributor>
    <dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/35965/3/Fakharuddin_0-372166.pdf"/>
    <dcterms:issued>2016-09-06</dcterms:issued>
    <dc:creator>Schmidt-Mende, Lukas</dc:creator>
    <dc:creator>De Rossi, Francesca</dc:creator>
    <bibo:uri rdf:resource="https://kops.uni-konstanz.de/handle/123456789/35965"/>
    <dc:contributor>Jose, Rajan</dc:contributor>
    <dc:creator>Fakharuddin, Azhar</dc:creator>
    <dc:creator>Watson, Trystan M.</dc:creator>
    <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2016-11-18T13:49:41Z</dc:date>
    <dc:creator>Jose, Rajan</dc:creator>
    <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/>
    <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
    <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2016-11-18T13:49:41Z</dcterms:available>
    <dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/35965/3/Fakharuddin_0-372166.pdf"/>
    <dc:contributor>Watson, Trystan M.</dc:contributor>
    <dc:language>eng</dc:language>
    <dcterms:rights rdf:resource="http://creativecommons.org/licenses/by/4.0/"/>
    <dc:contributor>Schmidt-Mende, Lukas</dc:contributor>
    <dcterms:abstract xml:lang="eng">Perovskite solar cells (PSCs) marked tremendous progress in a short period of time and offer bright hopes for cheap solar electricity. Despite high power conversion efficiency &gt;20%, its poor operational stability as well as involvement of toxic, volatile, and less-abundant materials hinders its practical deployment. The fact that degradation and toxicity are typically observed in the most successful perovskite involving organic cation and toxic lead, i.e., CH&lt;sub&gt;3&lt;/sub&gt;NH&lt;sub&gt;3&lt;/sub&gt;PbX&lt;sub&gt;3&lt;/sub&gt;, requires a deep understanding of their role in photovoltaic performance in order to envisage if a non-toxic, stable yet highly efficient device is feasible. Towards this, we first provide an overview of the basic chemistry and physics of halide perovskites and its correlation with its extraordinary properties such as crystal structure, bandgap, ferroelectricity, and electronic transport. We then discuss device related aspects such as the various device designs in PSCs and role of interfaces in origin of PV parameters particularly open circuit voltage, various film processing methods and their effect on morphology and characteristics of perovskite films, and the origin and elimination of hysteresis and operational stability in these devices. We then identify future perspectives for stable and efficient PSCs for practical deployment.</dcterms:abstract>
    <dc:contributor>De Rossi, Francesca</dc:contributor>
    <dcterms:title>Research Update : Behind the high efficiency of hybrid perovskite solar cells</dcterms:title>
    <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
  </rdf:Description>
</rdf:RDF>
Interner Vermerk
xmlui.Submission.submit.DescribeStep.inputForms.label.kops_note_fromSubmitter
Kontakt
URL der Originalveröffentl.
Prüfdatum der URL
Prüfungsdatum der Dissertation
Finanzierungsart
Kommentar zur Publikation
Allianzlizenz
Corresponding Authors der Uni Konstanz vorhanden
Internationale Co-Autor:innen
Universitätsbibliographie
Ja
Begutachtet
Diese Publikation teilen