@article{Kim2004Relax-5246,
  year={2004},
  doi={10.1103/PhysRevB.70.035421},
  title={Relaxation dynamics of magic clusters},
  volume={70},
  journal={Physical Review / B},
  author={Kim, Young Dok and Niemietz, Marco and Gerhardt, Peter and Gynz-Rekowski, Felix von and Ganteför, Gerd},
  note={Article Number: 35421}
}

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    <dc:contributor>Gerhardt, Peter</dc:contributor>
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    <dcterms:title>Relaxation dynamics of magic clusters</dcterms:title>
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    <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T14:54:19Z</dc:date>
    <dc:creator>Niemietz, Marco</dc:creator>
    <dcterms:bibliographicCitation>First publ. in: Physical Review / B 70 (2004), 035421</dcterms:bibliographicCitation>
    <dc:creator>Gerhardt, Peter</dc:creator>
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    <dcterms:abstract xml:lang="eng">Using femtosecond time-resolved two-photon photoemission spectroscopy, relaxation rates of the optically excited states in Al13− , Si4− , and Au6− clusters are estimated to be 250  fs , 1.2  ps , and about 1  ns , respectively. These clusters show closed electronic shell structures and large gaps between the highest occupied molecular orbital and the lowest unoccupied molecular orbital in the anionic (Al13−) or neutral ( Si4  and Au6 ) states. Thus the different behaviors of these clusters for the relaxation dynamics cannot be rationalized within a relaxation mechanism dominated by Auger-like electron-electron coupling. We suggest that for these small clusters, the major decay mechanism might be electron-phonon coupling.</dcterms:abstract>
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